Selective nitrogen doping in graphene for oxygen reduction reactions.

نویسندگان

  • Satoshi Yasuda
  • Li Yu
  • Jeheon Kim
  • Kei Murakoshi
چکیده

Nitrogen-doped graphene materials with abundant pyridinic and quaternary nitrogen species were selectively synthesized by thermal surface polymerization of nitrogen-containing aromatic molecules. Catalytic studies revealed that the oxygen reduction by nitrogen-doped graphene, containing pyridinic and quaternary nitrogen species, proceeds via a four- and two-electron reduction pathway, respectively, in alkali-based solutions.

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عنوان ژورنال:
  • Chemical communications

دوره 49 83  شماره 

صفحات  -

تاریخ انتشار 2013